Select the most appropriate option that can substitute the underlined segment in the given sentence: No sooner did Mr. Piyahri Mishra finish his chemistry lecture that the students began to leave.

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The phrase 'No sooner ... than ...' is a correlative conjunction used to indicate that one event happened immediately after another. The correct conjunction to use after 'No sooner' is 'than', not 'that', 'then', 'so', or 'and'. Therefore, the correct substitution is 'than the students began to leave.'

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